Search results for "Spectroscopie résolue en temps"
showing 2 items of 2 documents
Controlling rotational dynamics of molecules by shaped ultra-short laser pulses
2004
This manuscript presents various studies falling under the set of themes of coherent control. We establish, as well theoretically as in experiments, the possibility of finely handling the rotational dynamics of linear molecules. In order to operate this handling, the ultra-short pulses are shaped by a pulse shaper. Its principle and its installation are described in a detailed way. The rotational dynamics of the linear nitrogen molecule (N2) is handled while exploiting the relative excitation between the even and odd rotational components of the wavepacket in weak mode of field. That, we chose a periodic phase modulation well defined of the exiting pulse. A temporal analysis comes to clarif…
Cavités plasmoniques et nanosources optiques
2013
Optical microcavities exhibit high resonance quality, so that, they are of key interest for the design of low-threshold lasers or for achieving strong coupling regime. But, such systems support modes whose the volume remain diffraction limited.In this manuscript, we are interested in their plasmonic counterparts because they support confined modes at the sub-wavelength scale. First, we study an in-plane plasmonic cavity which is the transposition of 1D optical cavity to surface wave. We characterize the cavity by measuring the fluorescence lifetime of dye molecules deposited inside.Then, we are interested in 3-dimension mode confinement achieved by spherical metal nanoparticles. We discuss …